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The first example of a catalytic asymmetric vinylogous Povarov reaction is presented. 1-N-Acylamino-1,3-butadienes react selectively at their terminal double bond in the presence of a chiral phosphoric acid catalyst, delivering highly enantioenriched 1,2,3,4-tetrahydroquinolines bearing a synthetically versatile enecarbamate group at the 4-position.


Lorenzo Caruana, Mariafrancesca Fochi, Silvia Ranieri, Andrea Mazzanti, Luca Bernardi. Catalytic highly enantioselective vinylogous Povarov reaction. Chemical communications (Cambridge, England). 2013 Jan 30;49(9):880-2

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PMID: 23238127

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